Acta Physica Polonica A
Vol. 97 No 3 March 2000
 
CHEMICAL POTENTIAL AS A DETECTOR OF PHASE TRANSITIONS IN SOLIDS

M. Matlaka, E. Goslawskaa, B. Grabieca and Kh. Eidb

a Institute of Physics, Silesian University, Uniwersytecka 4, 40-007 Katowice, Poland
b Physics Department, Faculty of Education, Ain-Shams University, Roxy, Cairo, Egypt

We show that the chemical potential exhibits small but distinct kinks at all critical temperatures as the evidence for phase transitions in the electronic system, structural phase transitions included. In the case of, at least, two kinds of interacting electrons average occupation numbers exhibit the same behavior.
 
PACS numbers: 74.70.-b, 75.30.Kz, 75.40.Cx
 
SUPERCONDUCTING AND MAGNETIC PHASES WITH 1212-TYPE OF STRUCTURE

E.P. Khlybova,b, I.E. Kostylevab, K. Nenkova ,c, V.I. Nizhankovskiia, T. Palewskia and J. Warchulskaa

a International Laboratory of High Magnetic Fields and Low Temperatures Gajowicka 95, 53-421, Wroclaw, Poland
b Institute of High Pressure Physics, 142092 Troitsk Moscow reg, Russia
c Institut fur Festkörper- und Werkstofforschung Dresden P.O.Box 270016, 01171 Dresden, Germany

Studies of magnetic and transport properties of the 1212 compounds MA'2A''Cu2O7-x (M 3D Al or Tl; A'= Sr or Ba; A''= RE, Y, and Ca) revealed a number of interesting magnetic phenomena. Apart from high-temperature superconductivity, these compounds exhibit spontaneous antiferromagnetism, field induced antiferromagnetism or ferromagnetism. The different magnetic orders and superconductivity may be realized in the same compound as a result of the phase separation.
 
PACS numbers: 74.25.Ha, 74.72.Jt
 
COMPARISON OF FLUX PINNING IN SINGLE CRYSTALS AND MELT-TEXTURED YBa2Cu3O7-x

R. Puzniak1, A. Wisniewski1, M. Baran1 and L. Zhou2


1 Institute of Physics, Polish Academy of Sciences Al. Lotników 32/46, 02-668 Warsaw, Poland 2Northwest Institute for Nonferrous Metal Research, Xi'an, P.R. China

Flux pinning properties of single crystals and melt-textured samples of YBa2Cu3O7-x were studied for external magnetic field oriented parallel and perpendicular to the CuO2 planes (ab-planes). For H || ab vortex behaviour is mainly determined by a very effective intrinsic pinning mechanism. The irreversibility line is located in the region of higher fields and temperatures in comparison with the irreversibility line for H perp ab. In a single crystal for H\perp ab, we observed an increase in the critical current density jc with magnetic field - the so-called ``fishtail effect'' - in a very broad temperature range. For H || ab, this effect is observed only at temperatures close to Tc, when the intrinsic pinning is much weaker.
 
PACS numbers: 74.60.Ge, 74.60.Jg, 74.72.Bk
 
LIEB-MATTIS MODEL FOR TWO INTERPENETRATING ANTIFERROMAGNETS

D. Schmalfuss, S.E. Krüger and J. Richter

Institut für Theoretische Physik, Universität Magdeburg PF 4120, 39016 Magdeburg, Germany

We investigate a frustrated Lieb-Mattis-like spin-1/2 model that is a reference model for the corresponding square-lattice Heisenberg model describing the unusual magnetic properties of Ba2Cu3O4Cl2. Due to frustration we obtain a rich magnetic phase diagram. We find two critical temperatures in accordance with recent experiments on Ba2Cu3O4Cl2.
 
PACS numbers: 75.10.Jm
 
CORRELATION INDUCED OPTIMIZATION OF WAVE FUNCTIONS: THE HUBBARD CHAIN

J. Spalek, R. Podsiadly

Marian Smoluchowski Institute of Physics, Jagiellonian University Reymonta 4, 30-059 Kraków, Poland

and W. W&oacutejcik

Institute of Physics, Tadeusz Kosciuszko Technical University Podchorazych 1, 30-084 Kraków, Poland

We determine the explicit form of the single-particle Wannier functions {wi(r)} appearing in the parameters of quantum models. The method is illustrated on the example of the Hubbard chain, for which we derive the renormalized wave equation starting from a variational principle and by treating the system ground state energy as a functional of {wi(r)} and their derivatives. In this manner, the optimized basis is obtained only after the electronic correlations have been included in the rigorous Lieb-Wu solution. The results for the ground state energy and the size of the renormalized s-type orbitals, both as a function of interatomic distance, are calculated explicitly.
 
PACS numbers: 71.10.Fd, 71.15.Fv, 31.25.Nj
 
COQBLIN-SCHRIEFFER IMPURITY WITH LOCAL EXCHANGE COUPLING: A PERTURBATIVE APPROACH

P. Stefański

Institute of Molecular Physics, Polish Academy of Sciences Smoluchowskiego 17, 60-179 Poznań, Poland

The Coqblin-Schrieffer one-impurity model with the additional local exchange interaction is studied within diagrammatic approach. The Ruderman-Kittel-Kasuya-Yoshida-type local exchange interaction between f electrons of the impurity and a channel of conduction electron l=0 partial waves is treated in the molecular field approximation. The perturbation expansion resummation for the Coqblin-Schrieffer hybridization mediated interaction vertex part is carried out in the ladder approximation yielding the formula for the Kondo temperature TK decreasing with increased local exchange. Moreover, the temperature divergence of the susceptibility at TK is shifted towards T=0. For some critical strength of the local exchange interaction the susceptibility approaches a Curie-type dependence as for an uncompensated impurity magnetic moment. A relation to the ``Kondo disorder'' model, which leads to the non-Fermi-liquid behavior, is discussed.
 
PACS numbers: 71.10.Hf, 71.20.Eh, 72.15.Qm, 75.20.Hr
 
STUDY OF COMPOSITES CONSISTING OF HIGH-Tc SUPERCONDUCTOR AND FINE MAGNETIC PARTICLES

M. Timkoa, P. Kopcanskya, J. Kovavca, M. Konerackaa and V. Plechacekb

a Institute of Experimental Physics, Slovak Academy of Sciences Watsonova 47, 043 53 Kosice, Slovak Republic
b Institute of Physics, Czech Academy of Sciences Cukrovarnicka 10, 162 00 Praha 6, Czech Republic

The composite systems as a mixture of fine magnetic particles of Fe3O4 and superconducting powder such as Bi1.8Pb0.2Sr2Ca2Cu3O10+x were prepared. The influence of internal magnetic field (generated by magnetic particles) on the superconducting properties of prepared composites were studied as a function of concentration of magnetic particles and their magnetic state. The observed data both of the shielding and the Meissner effect were compared with corresponding linear combination of pure signals of magnetite and superconductor, respectively. The large differences were observed for demagnetized samples. It means that result must be discussed in the frame of the distribution of internal magnetic field created by the magnetic particles.
 
PACS numbers: 74.72.Hs, 75.50.Tt
 
PHASE FLUCTUATIONS AND BCS-LP CROSSOVER IN 2D SHORT COHERENCE LENGTH SUPERCONDUCTORS

B. Tobijaszewska and R. Micnas

Institute of Physics, A. Mickiewicz University Umultowska 85, 61-614 Poznań, Poland

We study the effects of phase fluctuations in 2D short-coherence length superconductors on the basis of the extended Hubbard model with intersite attraction. In the Kosterlitz-Thouless scenario the critical temperatures for anisotropic pairings were determined and compared with the ones from BCS Hartree-Fock approximation. The Uemura-type plots, i.e. the critical temperature vs. zero temperature phase stiffness, were obtained for extended s-wave and dx2-y2-wave pairings. We also discuss the crossover from BCS to local pair superconductivity for d-wave pairing.
 
PACS numbers: 74.20.-z, 71.10.Fd, 74.20.Fg, 74.20.Mn, 74.72.-h
 
TRANSPORT PROPERTIES OF THE U1-xThxPt SYSTEM

V.H. Tran and R. Troc

W. Trzebiatowski Institute of Low Temperature and Structure Research Polish Academy of Sciences, P.O. Box 1410, 50-950 Wroclaw, Poland

We present the results of measurements of electrical resistivity (rho(T)) and magnetoresistance (Delta varrho varrho0(T)) on the solid solutions U1-xThxPt (x=0-0.8). The Curie temperature (Tc=21 K) found for the parent compound UPt, is steadily reduced upon the Th-substitution. The rho(T) and Delta varrho varrho0(T) functions provide evidence of electron scattering due to spin fluctuations. The most interesting feature of Delta varrho varrho0 is its high value of about -22% found for UPt and U0.9Th0.1Pt at their Tc and B=8 T. For samples with x >= 0.2, the value of Delta varrho varrho0 at 4 K and 8 T increases with x and becomes positive for Th-composition x >= 0.6.
 
PACS numbers: 72.15.Eb, 72.15.Gd, 75.70.Pa
 
DESTRUCTION OF ANTIFERROMAGNETIC ORDER BY LOCALIZED POLARONS

Z. Wilamowski and E.M. Hankiewicz

Institute of Physics, Polish Academy of Sciences Al. Lotników 32/46, 02-668 Warszawa, Poland

Analysis of a finite spin cluster indicates a possibility of the formation of purely magnetic polarons in low-dimensional antiferromagnets. It is shown that for parameters characteristic of CuO2 based superconductors a strong antiferromagnetic polaron can occur. The destruction of antiferromagnetic order by the presence of a magnetic polaron is discussed.
 
PACS numbers: 74.20.-z, 75.10.-b, 74.20.Mn
 
THE REMARK ABOUT AN ANALOGY BETWEEN MAGNETOCALORIC BEHAVIOUR OF TYPE II SUPERCONDUCTORS AND FERROMAGNETIC MATERIALS

Z. Kalva and P. Manek

Center for Theoretical Study, Charles University and the Academy of Sciences Jilska 1, 11000 Praha 1, Czech Republic

The analogy between magnetocaloric behaviour of type II superconductors and anisotropic ferromagnetic materials is discussed. Special attention is devoted to the influence of anisotropy on the negative magnetocaloric effect near phase transitions.
 
PACS numbers: 75.30.Sg, 74.60.Ge
 
THERMODYNAMICS OF PSEUDOSPIN-ELECTRON MODEL IN THE U=0 LIMIT

I.V. Stasyuk, A.M. Shvaika and K.V. Tabunshchyk

Institute for Condensed Matter Physics, National Academy of Sciences of Ukraine 1 Svientsitskii Str., 290011 Lviv, Ukraine

Analytical consideration of a pseudospin-electron model in the absence of electron correlations is presented. Pseudospin and electron number mean values, thermodynamic potential, pair correlation functions are obtained in the same self-consistent approximation. The possibility of either first or second order phase transitions between different uniform phases (bistability) as well as between the uniform and the chessboard one is shown. In the regime n={const}, an instability with respect to phase separation can take place.
 
PACS numbers: 71.10.Fd, 71.38.+i, 77.80.Bh, 63.20.Ry
 
THEORETICAL STUDY OF PHASE DIAGRAMS FOR REENTRANT SUPERCONDUCTING Er1-xHoxX, Er1-xGdxX, Er1-xTmxX, Ho_ xLu1-xX, AND Sm1-xErxX (X = Rh_4B_4) ALLOYS

E. Gos/lawska and M. Matlak

Institute of Physics, Silesian University, Uniwersytecka 4, 40-007 Katowice, Poland

We consider a simplified version of the s{-}f model, supplemented by the intersite Cooper pairs interaction between conduction electrons with opposite spins to investigate ferromagnetic and superconducting properties of an alloy Re1-x(1)Rex(2)X (Re(1),(2) - rare earth elements, X = Rh4B4) using the virtual crystal approximation. For a suitable choice of the model parameters we can reproduce the phase boundaries of the experimentally measured phase diagrams for Er1-xHoxX, Er1-xGdx X, Er1-xTmxX, HoxLu1-xX, and Sm1-xErxX alloys.
 
PACS numbers: 75.30.Kz, 75.40.Cx
 
LOW TEMPERATURE TRANSPORT AND MAGNETIC PROPERTIES OF SmB6

S. Gabania, K. Flachbartb, V. Pavlikb, E. Konovalovac, Y. Padernoc and T. Herrmannsdörferd

a Department of Experimental Physics, P.J. Safarik University Park Angelinum 9, 04154 Kosice, Slovakia
b Institute of Experimental Physics, SAS, 04353 Kosice, Slovakia
c Institute for Problems of Materials Science, UAS, 252680 Kiev, Ukraine ^d Physikalisches Institut, Universität Bayreuth, 95440 Bayreuth, Germany

We present results of transport and magnetic properties of three single-crystalline samples of the intermediate valence small-gap semiconductor SmB6 at low temperatures. The received resistivity dependences of the samples below 0.5 K exhibit an activated behavior with an energy gap of a few mK. The temperature dependences of the magnetic susceptibility show an increase below 15 K which can be accounted for by impurities, by bare Sm3+ ions or by a small amount of in-gap magnetic 4f55d1 states.
 
PACS numbers: 75.20.Hr, 71.28.+d
 
CURRENT FLUCTUATIONS IN FERROMAGNETIC TUNNEL JUNCTIONS

B.R. Bulkaa, J. Martineka, G. Michaleka and J. Barnasb

a Institute of Molecular Physics, Polish Academy of Sciences Smoluchowskiego 17, 60-179 Poznań, Poland ^bDepartment of Physics, A. Mickiewicz University Umultowska 85, 61-614 Poznań, Poland

Current shot noise in a double junction consisting of a small metallic grain connected to two ferromagnetic electrodes is analysed in the limit of sequential tunneling. We show that, apart from charge fluctuations, there are strong spin fluctuations. We also show that two distinct relaxation processes can be distinguished in the frequency dependent current noise: one in a low frequency range and corresponding to spin fluctuations and another one in a high frequency range corresponding to charge fluctuations.
 
PACS numbers: 75.70.Pa, 73.50.Td, 73.23.Hk, 73.40.Gk
 
CORRELATIONS OF MECHANICAL STRESSES AND MAGNETICAL BEHAVIOUR OF ION IMPLANTED MAGNETO-OPTICAL LAYERS

F. Hubenthal and K. Röll

University of Kassel, Heinrich-Plett Str. 40, 34132 Kassel, Germany

Magneto-optical materials such as TbFeCo are used for data storage in a wide range. Especially the perpendicular magnetic anisotropy is necessary for high density recording. But the origin of the perpendicular magnetic anisotropy in these magneto-optical layers is not exactly known. In our experiments magneto-optical layers were implanted with heavy ions, with the aim to change the magnetic behaviour of these layers. After the implantation there is a dramatical change in the magnetical and mechanical behaviour, too.
 
PACS numbers: 61.72.Ww
 
MAGNETIC STRUCTURES IN ULTRATHIN FILMS AND NANOSTRUCTURES: SIMULATION

J.-C.S. Levya, A. Ghazalib and E.Yu. Vedmedenkoc

a LPTMC, case 7020, Universite Paris 7, 75251 Paris 5, France
bGPS, UMR-7588 CNRS, Universites Paris 7 et Paris 6, 75251 Paris 5, France
cMPI fšr Mikrostrukturphysik, 06120 Halle, Germany

In magnetic ultrathin films and dots, competing exchange, anisotropy and dipolar couplings lead to a large variety of magnetic structures. These structures are obtained by means of the Monte Carlo simulations. Three classes of magnetic structures are obtained according to anisotropy-to-dipolar energy ratio: Ising striped structures, XY-spin structures with vortices, and twisted spin phases at the spin = reorientation transition. Domain wall nucleation and motion at the coercive field are also accessible.
 
PACS numbers: 75.70.Ak, 75.50.Tt, 75.60.Ch, 75.40.Mg
 
MAGNETIC ANISOTROPY IN EuS-PbS MULTILAYERS

T. Storya, C.H.W. Swüsteb, H.J.M. Swagtenb, W.J.M. de Jongeb, A. Stachow-Wójcikc, A. Twardowskic, M. Arciszewskaa, W. Dobrowolskia, R.R. Galazkaa and A.Yu. Sipatovd

a Institute of Physics, Polish Academy of Sciences Al. Lotników 32/46, 02-668 Warsaw, Poland
b Department of Physics, Eindhoven University of Technology 5600 MB Eindhoven, The Netherlands
c Institute of Experimental Physics, Warsaw University Hoza 69, 00-681 Warsaw, Poland
d Kharkov = State Polytechnical University, 21, Frunze Street, 310002 Kharkov, Ukraine

We present the results of ferromagnetic resonance studies of the thickness dependence of magnetic anisotropy in 2 series of EuS-PbS multilayers grown on (111) BaF2 and (100) KCl substrates with the EuS thickness varying in the range d=6-70 A. The anisotropy constant K was found to follow the dependence K(d)=KV+2KS/d , with the surface term KS larger for layers grown on BaF2 as compared to KCl. This difference is discussed in terms of different thermal stress-induced distortions of cubic crystal lattice of EuS. We found that the thickness of EuS layer required for the perpendicular (to the layer) magnetization is d <= 2-3 A, i.e., it is below 1 monolayer.
 
PACS numbers: 75.50.Pp, 75.70.Ak
 
MAGNETIC ANISOTROPY IN Co/Nd MULTILAYERS WITH DEPTH-SELECTIVELY INSERTED 57Fe PROBE LAYER

L.T. Baczewskia, K. Mibub, T. Nagahamab and T. Shinjob

a Institute of Physics, Polish Academy of Sciences Al. Lotników 32/46, 02-668 Warsaw, Poland
b Institute for Chemical Research, Kyoto University, Uji, Kyoto-fu, Japan

Multilayers of Co/Nd with probe layer of 2 AA of 57Fe evaporated in UHV conditions were studied by means of vibrating sample magnetometry and Mössbauer spectroscopy at T = 4.2 K. Isomer shift, hyperfine field distribution and direction was obtained from the Mössbauer data computer fitting. Magnetic anisotropy was studied and discussed. The easy magnetization direction was close to the perpendicular direction for both samples but the tendency to perpendicular anisotropy was stronger when the Fe probe layer was placed in the vicinity of Co/Nd interface.
 
PACS numbers: 75.30.Gw, 75.70.-i, 76.80.+y
 
TUNNELING MAGNETORESISTANCE IN PLANAR FERROMAGNETIC JUNCTIONS

M. Wilczyński and J. Barnas

a Institute of Physics, Warsaw Technical University Koszykowa 75, 00-662 Warszawa, Poland
b Department of Physics, Adam Mickiewicz University Umultowska 85, 61-614 Poznań, Poland

Bias dependence of the tunnel magnetoresistance in simple planar ferromagnetic junctions is considered theoretically within the one-band model. The limit of sequential tunnelling in double junctions with a non-magnetic central electrode is studied as well. In this case tunnel magnetoresistance exists only when the spin relaxation time due to spin-flip scattering processes inside the central electrode is sufficiently long.
 
PACS numbers: 72.15.Gd, 73.40.Gk, 75.70.-i
 
INFLUENCE OF FILM THICKNESS ON THE MICROSTRUCTURE AND MAGNETIC PROPERTIES OF FINEMETIC THIN FILMS

R. Dlugosa, P. Sovaka, J. Balcerskib, J. Füzera and P. Kollara

a Faculty of Science, P.J. Safarik University, Park Angelinum 9, 041 54 Kosice, Slovakia
b Department of Solid State Physics, University of L&oacutedz Pomorska 149/153, 90-236 Lódz, Poland

The aim of this work was to study the influence of film thickness on the structure and magnetic properties of finemetic thin films after annealing. Thin films with the various thickness (from 20 nm up to 700 nm) were prepared by DC sputtering method. The heat treatments of the films for further structural and magnetic observations were performed at the temperature range 300-500 oC for 15 min in vacuum furnace. Structural observations were carried out by transmission electron microscopy. Coercivity was determined from hysteresis loops traced with fluxmeter and Kerr magnetooptical hysteresisgraph. All the experimental results confirm a different magnetic behaviour of the thin films according to their thickness.
 
PACS numbers: 68.55.Jk, 73.50.Jt, 75.70.Ak
 
COMPLEX MAGNETIC STRUCTURE OF STRONGLY COUPLED Fe/Si MULTILAYERS

J. Dubowika, F. Stobieckia, B. Szymańskia, Yu.V. Kudryavtsevb, A. Grabiasc and M. Kopcewiczc

a Institute of Molecular Physics, Polish Academy of Sciences Smoluchowskiego 17, 60-179 Poznań, Poland
b Institute of Metal Physics, National Academy of Sciences of Ukraine Kiev-142, Ukraine ^cInstitute of Electronic Materials Technology, Wólczyńska 133, 01-919 Warsaw, Poland

Fe/Si multilayers with strong bilinear and biquadratic couplings were investigated. A complex structure revealed by the Mössbauer spectroscopy corresponds to multimode ferromagnetic resonance spectra in a non-saturated state. Simple dispersion relations for antiferromagnetic coupled bilayer structures are shown to be inapplicable to the Fe/Si multilayers with a strong biquadratic component to the antiferromagnetic bilinear coupling.
 
PACS numbers: 75.70.-i, 68.55.-a, 76.50.+g
 
INTERACTION BETWEEN MAGNETIC LAYERS IN STRUCTURES WITH NARROW-GAP IV-VI SEMICONDUCTORS

V.K. Dugaeva, V.I. Litvinova, W. Dobrowolskib and T. Storyb

a Chernovtsy Department of the Institute of Materials Science Problems Ukrainian Academy of Sciences, Vilde 5, 274001 Chernovtsy, Ukraine
b Institute of Physics, Polish Academy of Sciences Al. Lotników 32/46, 02-668 Warsaw, Poland

The results of calculation of the indirect exchange interaction between magnetic layers are presented for the case of a structure with narrow-gap semiconducting IV-VI quantum well. The main mechanism is a magnetic polarization of the size-quantized electrons and holes inside the well. This type of interaction is suggested for the explanation of recent experiments on EuS/PbS structures.
 
PACS numbers: 75.70.Cn, 75.50.Pp, 75.70.Ak
 
ROLE OF THE SURFACE ENERGY FOR THE FORMATION OF THE DOMAIN STRUCTURE AT MAGNETOELASTIC PHASE TRANSITION

H.V. Gomonaj and V.M. Loktev

National Technical University of Ukraine ``KPI'' 37, Ave. Peremogy, 252056, Kyiv, Ukraine

The formation of the domain structure during magnetic ordering in the pure antiferromagnet with the rotational (non-180o) domains can be treated as thermodynamically preferable if the free energy of the sample is minimized with the account of surface energy. The analogy between the role of magnetostatic energy in ferromagnets and surface energy of antiferromagnet is traced. The behavior of the domain structure and macroscopic strain tensor in the external magnetic field is investigated.
 
PACS numbers: 75.50.Ee, 75.60.Ch
 
MAGNETIC PROPERTIES OF IRON-BASED AMORPHOUS AND NANOCRYSTALLINE Fe-Zr-X-B (X: Cu, Al) ALLOY FILMS

I. Gosciańskaa, T. Tolińskib, H. Ratajczakb, P. Sovákc, R. Dlugosc and M. Koncc

a Institute of Physics, A. Mickiewicz University, Umultowska 85, 61-614 Poznań, Poland
b Institute of Molecular Physics, Polish Academy of Sciences Smoluchowskiego 17, 60-179 Poznań, Poland
c Department of Experimental Physics, P.J. Safarik University, Kosice, Slovakia

Thermal stability and magnetic properties of thin films, of a few Fe-based amorphous and nanocrystalline alloys, have been studied. The alloys belong to the class Fe-M-B, whose representatives are: Fe87Zr4Cu1B8, Fe87Zr7B6, and Fe87Zr7Al1B5 and are of particular interest because of their wide variety of magnetic properties. The films were prepared by flash evaporation onto liquid nitrogen cooled substrates. Measurements of the Kerr effect, the Hall effect, and ferromagnetic resonance in the films were carried out as functions of the annealing temperature. It was found that the changes in the coercive field Hc, resonance linewidth Delta Hpp, effective magnetization Meff, Hall parameters, and resistance were correlated with the structural changes in the studied films.
 
PACS numbers: 73.61.Tm, 75.50.Bb
 
PREISACH MAPS OF MULTILAYERED Co/Cu STRUCTURES

M. Gutowski, M.U. Gutowska, K. Piotrowski, L.T. Baczewski and A. Wawro

Institute of Physics, Polish Academy of Sciences Al. Lotników 32/46, 02-668 Warszawa, Poland

Magnetooptical Kerr effect measurements of room temperature hysteresis loops were taken using sandwich- and multilayer-type specimens and He-Ne laser light. For maximal external field of ~250 Gs the corresponding Kerr angle reached 0.04 deg. The samples were obtained in the Institute of Physics, Polish Academy of Sciences, Warszawa, using MBE method. The structure of samples may be described by a formula: substrate-buffer layer-(xCo/yCu)n -cover layer. Al2O3 (two orientations) and MgO were used as substrates, the buffer layer was made of W, Cu or Fe, x=15, 20 or 25 A, y=7, 8, 9, 10, 11, 12, 13, 14, and 20 Ć, n=25 and 30. 50 Ć of gold (Au) served as a cover layer. The genetic algorithm was subsequently used as a data processing tool, in order to reconstruct the Preisach map for each hysteresis loop. The diagrams clearly indicate changes of magnetic interactions caused by varying thicknesses of individual magnetic and non-magnetic layers.
 
PACS numbers: 75.40.Mg, 75.60.Ej, 75.70.-i, 78.20.Ls, 78.66.-w
 
COERCIVITY OF ULTRATHIN MAGNETIC FILMS WITH PERPENDICULAR ANISOTROPY

V. Zablotskiia, M. Kisielewskib, O. Tsiganenkoc and J. Ferred

a Physics Department, Donetsk State University, 340055 Donetsk, Ukraine
b Institute of Physics, University at Bialystok, Lipowa 41, 15-424 Bialystok, Poland
c Institute of Physics, Academy of Sciences of Czech Republic Na Slovance 2, 18040 Praha 8, Czech Republic
d Lab. de Phys. des Solides, URA CNRS 02, Université Paris-Sud, 91405 Orsay, France

The calculation of the temperature dependence of the domain wall coercivity of ultrathin magnetic films with perpendicular anisotropy is reported. In this case, the magnetization reversal is supposed to occur through domain wall motion. The proposed model takes into account thermal bending fluctuations of the domain wall, which is pinned by crystal defects such as grain boundaries. A fitting procedure, applied to recently published experimental data on the field induced domain wall velocity in Au/Co films, allows us to find out realistic values of the involved parameters.
 
PACS numbers: 75.60.-d, 75.60.Ch, 75.70.Ak
 
CREATION AND OBSERVATION OF DOMAIN STRUCTURES WITH A SPECIAL KERR MICROSCOPE

S. Knappmanna, K. Rölla and F. Stobieckib

a University Gh Kassel, Heinrich-Plett-Str. 40, 34132 Kassel, Germany
b Institute of Molecular Physics, Polish Academy of Sciences Smoluchowskiego 17, 60-179 Poznań, Poland

A Kerr microscope is presented, which on the one hand allows us to make, in a conventional manner, images of domains in thin films with perpendicular magnetic anisotropy. On the other hand, it is possible to heat the sample locally by a focussed laser beam and make images simultaneously. Therefore, it is possible to write domains thermomagnetically and further to observe temperature dependent magnetic reorientations. For demonstration domains have been created thermomagnetically in TbFe multilayers. Writing with low magnetic field leads to domains with a subdomain structure, as it has been found previously by Lorentz microscopy.
 
PACS numbers: 75.70.Kw
 
THE DISTRIBUTION OF MAGNETIZATION FOR A STEPPED FERRO-ANTIFERROMAGNET INTERFACE

O.K. Dudko and A.S. Kovalev

B. Verkin Institute for Low Temperature Physics and Engineering Ukrainian Academy of Sciences, 47 Lenin Avenue, 310164 Kharkov, Ukraine

Magnetization distribution of a disclination type connected with the atomic step on the ferro-antiferromagnet boundary is studied. The results are generalized for the periodic stepped interface.
 
PACS numbers: 75.30.Kz
 
THE EMERGENCE OF SUBSURFACE SPIN-WAVES IN FCC (110) MAGNETIC FILMS

S. Mamicaa, H. Puszkarskib and J.C.S. Lévyb

a Surface Physics Division, Faculty of Physics, Adam Mickiewicz University Umultowska 85, 61-614 Poznań, Poland
b Laboratoire de Physique Théorique de la Mati\egrave;re Condensée Université Paris 7-Denis Diderot, 2 Place Jussieu, 75221 Paris Cedex 05, France

We show that the emergence of subsurface branches in the spin-wave spectra of thin films is due to the deficiency of interactions with next-nearestneighbours, the position vectors of which are oblique to the film surface.
 
PACS numbers: 75.70.-i, 75.40.Gb, 75.30.Ds
 
SPONTANEOUS SURFACE MAGNETISATION OF SINGLE CRYSTAL MnF2 IN THE ANTIFERROMAGNETIC STATE

V.I. Nizhankovskiia, A.I. Khar'kovskiia and A.J. Zaleskib

a International Laboratory of High Magnetic Fields and Low Temperatures Gajowicka 95, 53-421 Wroclaw, Poland
b Institute of Low Temperature and Structural Research, Polish Academy of Sciences P.O. Box 937, 50-950 Wroclaw, Poland

Spontaneous magnetisation of (100) and (010) surfaces of a MnF2 single crystal in the antiferromagnetic state is discovered. A sign of the surface magnetisation is determined by a difference in dielectric constants varepsilon of MnF2 and ambient matter: magnetisation is directed to the substance with a smaller varepsilon.
 
PACS numbers: 75.30.Pd, 75.25.+z, 75.50.Ee
 
MAGNETIC ANISOTROPY OF NiMn/Ni AND NiMn/Cu/Ni THIN FILMS

T. Ogawa and T. Sato

Department of Instrumentation Engineering, Faculty of Science and Technology Keio University, 3-14-1 Hiyoshi, Kohoku-ku, Yokohama, Kanagawa 223-8522, Japan

The magnetic anisotropy of reentrant spin glass NiMn thin film, in the vicinity of the ferromagnetic Ni film, is investigated using NiMn/Ni, Cu/Ni/Cu (t=10 Ć and 500 Ć)/NiMn and NiMn/Ni/Cu (t=10 div 5000  Ć)/Ni films. The unidirectional anisotropy field of NiMn layer in NiMn/Ni film is smaller than that of bulk NiMn. In Cu/Ni/Cu (t=10 Ć and 500 Ć)/NiMn film, the unidirectional anisotropy field is almost independent of the Cu spacer thickness. These results can be explained in terms of magnetic coupling between the magnetic layers in addition to the film structure of NiMn layer.
 
PACS numbers: 75.30.Gw, 75.50.Lk, 75.70.Ak
 
CORRELATED ROUGHNESS EFFECTS IN THE GIANT MAGNETORESISTANCE OF MAGNETIC MULTILAYERS

G. Palasantzasa, J. Barnasb and J.Th.M. De Hossona

a Department of Applied Physics, Materials Science Center and Netherlands Institute for Metals Research University of Groningen, Nijenborgh 4, 9747 AG Groningen, The Netherlands
b Department of Physics, Adam Mickiewicz University Umultowska 85, 61-614 Poznań, Poland

Interface roughness effects on the giant magnetoresistance in magnetic multilayers are analysed theoretically for structures with non-conformal correlated interfaces. The roughness of each interface is described in terms of the K-correlation model and is characterized by the roughness exponent H(0<=H<1), correlation length xi, and rms roughness amplitude Delta. Coherent scattering by different interfaces is also taken into account.
 
PACS numbers: 72.15.Gd, 73.40.Jn
 
EDGE PINNING EFFECTS AND GIANT THERMAL INSTABILITY OF MAGNETIZATION HYSTERESIS LOOPS IN THIN NANO-SCALE MAGNETS

A.F. Popkova, L.L. Savchenko^b and N.V. Vorotnikovac

a Zelenograd Research Institute of Physical Problems Zelenograd, 103575 Moscow, Russia
b Physical Department, Moscow State University Vorobjevy Gory, 119899 Moscow, Russia ^cInstitute of Physics and Technology, Russian Academy of Science Nakhimovsky avenue 34, 117218 Moscow, Russia

Magnetization reversal modes of super-thin nano-scale particles with a high magnetization and low anisotropy are analyzed by solving magnetic moment motion equations. A new kind of thermal hysteresis instability connected with the random mutual transformation of the main magnetization modes is predicted by simulations.
 
PACS numbers: 75.60.Ej, 67.80.Jd
 
SPIN-WAVE RESONANCE IN THE FeBr2 METAMAGNETIC THIN FILM

W. Rudziński

Faculty of Physics, Adam Mickiewicz University Umultowska 85, 61-614 Poznań, Poland

The spin-wave resonance in the thin FeBr2 field-induced metamagnet in the paramagnetic phase with the (001) surfaces and at low temperatures is examined theoretically. It is found that the absorption spectrum is strongly affected by modifications of the surface exchange parameters. Also, the conditions for the appearance of various surface and bulk spin-wave features are discussed.
 
PACS numbers: 75.30.Ds, 75.70.Ak
 
MAGNETISATION OF Co/Ti MULTILAYERS

K. Smardza, L. Smardzb and A. Jezierskib

a Inst. of Mater. Sci. and Eng., University of Technology Pl. Curie 5, 60-965 Poznań, Poland
b Institute of Molecular Physics, Polish Academy of Sciences Smoluchowskiego 17, 60-179 Poznań, Poland

We studied experimentally and theoretically the magnetisation of the Co/Ti multilayers. The results showed that the magnetic moments on Co atoms located at the Co-Ti interface are strongly reduced. For dTi=0.35 nm the estimated effective non-magnetic Co thickness at the Co-Ti interface amounts approx 0.08 nm and approx 0.1 nm at 4 K and 295 K, respectively. We found a good agreement between experimentally determined and theoretically calculated magnetisations.
 
PACS numbers: 75.70.-i, 75.30.Et
 
MAGNETIC PROPERTIES OF NANOCRYSTALLINE Co/Ti AND Co/Zr MULTILAYERS

L. Smardza and K. Smardzb

a Institute of Molecular Physics, Polish Academy of Sciences Smoluchowskiego 17, 60-179 Poznań, Poland
b Institute of Mater. Sci. and Eng., University of Technology Pl. Curie 5, 60-965 Poznań, Poland

It is shown that the Co sublayers grow in the soft magnetic nanocrystalline phase up to a critical thickness dapprox3 and 2.8 nm for Co/Ti and Co/Zr MLs, respectively. The rapid decrease in the interlayer exchange coupling could be explained by its strong damping due to formation of a non-magnetic quasi-amorphous Co-Ti and Co-Zr alloy layer at the interfaces. The nanocrystalline 2.2 nm-Co/2 nm-Ti ML shows a weak 90° coupling near the transition zone from ferromagnetic to zero coupling.
 
PACS numbers: 75.70.-i, 75.30.Et
 
MAGNETIC AND ELECTRIC TRANSPORT PROPERTIES OF Fe-Hf-O FILMS PREPARED BY SUPERSONIC PLASMA JET METHOD

V. Soyka, L. Kraus, Z. Frait, M. Sicha and L. Jastrabik

Institute of Physics, ASCR, Na Slovance 2, 18221 Praha 8, Czech Republic

The influence of deposition conditions on the structure, magnetic properties, and electrical resistivity of Fe-Hf-O films, prepared by the supersonic plasma jet deposition technique, was investigated. Composition of the films was controlled by the nozzle composition and the working gas. It varied in the limits: 15-68 at.% of Fe, 0.5-8 at.% of Hf and 29-80 at.% of O. The films were mainly X-ray amorphous. Some of them showed a weak and broad peak near the [110] reflection of alpha-Fe indicating the presence of Fe-rich clusters in an amorphous matrix. Depending on the deposition parameters the magnetic properties vary from paramagnetic to ferromagnetic ones. The electrical resistivity changes from the metallic to the hopping type. In some samples a large negative magnetoresistance is observed.
 
PACS numbers: 75.50.Kj, 75.70.Pa
 
HYPERFINE FIELD IN YIG WITH CHARGED SUBSTITUTION

J. Kohouta, H. Stepánkováa, J. Englicha, P. Novákb, M. Kuceraa and K. Nitschb

a Faculty of Mathematics and Physics, Charles University 180 00 Prague 8, V Holesovickách 2, Czech Republic ^bInstitute of Physics, Academy of Sciences Cukrovarnická 10, 16 253 Prague 6, Czech Republic

57Fe NMR spectra were measured on thin films of yttrium iron garnet with divalent (Ca2+) and tetravalent (Ge^{4+}) cation substitutions using the spin echo technique at 4.2 K. A series of Y3-xCaxFe5-xGexO12 samples with 0 <= x <= 0.0 5 was prepared by an epitaxial growth from BaO/B2O3/BaF2 flux on gadolinium gallium garnet substrate. Satellite lines corresponding to the iron ions having the Ge4+ and Ca2+ in their neighbourhood were identified. The sample with the germanium content of x(Ge) = 0.004 and (110) substrate orientation was used for a detailed study: NMR spectra of this sample were measured in an external magnetic field of 0.1 T applied along several directions in the plane of the film. The modification of the isotropic part and the anisotropy tensor of the hyperfine interaction caused by the Ge4+ substituent were obtained from the experimental data. The results were compared with those previously reported for trivalent substitution (Ga3+).
 
PACS numbers: 76.60.-k, 75.50.Gg
 
TEMPERATURE DEPENDENCE OF MAGNETISATION REVERSAL AND GMR IN SPIN VALVE STRUCTURES

F. Stobieckia, T. Stobieckib, B. Ockerc, W. Maassc, W. Powroznikb, A. Pajad, C. Loche and K. Rölle

a Institute of Molecular Physics, Polish Academy of Sciences Smoluchowskiego 17, 60-179 Poznań, Poland
b Department of Electronics, University of Mining and Metallurgy, Krak/ow, Poland ^cBalzers Process Systems GmbH, Alzenau, Germany
d Department of Solid State Physics, Faculty of Physics and Nuclear Techniques University of Mining and Metallurgy, Kraków, Poland
e Department of Physics, University of Kassel, Germany

Temperature measurements of magnetisation reversal, resistance and magnetoresistance of Co/Cu/Co/FeMn spin valve structures deposited in different conditions were performed. The influence of exchange anisotropy energy, interlayer coupling energy, and electron transport properties were taken into consideration in explaining differences in giant magnetoresistance effect of investigated samples.
 
PACS numbers: 75.70.Pa, 68.55.Ln, 68.55.-a
 
THE IMPROVEMENT OF ATOMIC FORCE MICROSCOPE SUITABLE FOR MAGNETIC DOMAIN STRUCTURE MEASUREMENTS

I. Sveklo, W. Dobrogowski, M. Kisielewski and A. Maziewski

Institute of Physics of Bialystok University, Lipowa 41, 15-424 Bialystok, Poland

Based on commercial Burleigh METRISTM-2000 Atomic Force Microscope two methods of magnetic force measurements were realised. The developed system was successfully applied for study of magnetic structure of both YIG-garnet and CoNi/Pt magneto-optic multilayers.
 
PACS numbers: 75.70.-i, 75.30.Pd, 61.16.Ch
 
DIPOLAR CONTRIBUTIONS TO MAGNETOELASTIC ENERGY OF CRYSTAL GRAINS WITH INTERFACES

T. Szumiataa, R. Zuberekb, H. Szymczakb and J. Gonzalezc

a Department of Physics, Technical University of Radom Malczewskiego 29, 26-600 Radom, Poland
b Institute of Physics, Polish Academy of Sciences Al. Lotników 32/46, 02-668 Warsaw, Poland
c Departamento de Fisica de Materiales, Universidad del Pais Vasco Paseo Manuel de Lardizabal, 3, 20009 San Sebastian, Spain

The magnetic anisotropy and magnetostriction in nanocrystalline grains in non-magnetic or magnetic matrix (nanoparticles or nanocrystalline materials) differ from their bulk properties. The interactions between atoms at the interface play the important role in these magnetic properties. In this paper the magnetic dipolar contribution to magnetostriction energy has been calculated for spherical crystal grains (of bcc and fcc symmetry) with interface layer of atoms possessing different magnetic moment. Total magnetoelastic energy of the sphere-interface system is a sum of magnetoelastic energy of the sphere, energy of the interactions between the sphere and the interface and also the energy of the interface. It was shown that magnetoelastic energy depends on the sphere size and interface thickness.
 
PACS numbers: 75.80.+q, 68.90.+g, 78.66.Jg
 
MAGNETIC PROPERTIES AND GMR OF SPUTTERED PERMALLOY/Au MULTILAYERS

B. Szymański and F. Stobiecki

Institute of Molecular Physics, Polish Academy of Sciences Smoluchowskiego 17, 60-179 Poznań, Poland

We report on structural, magnetic, and GMR properties of permalloy/Au multilayers where permalloy = Ni83Fe17, deposited by face-to-face sputtering onto Si(111) substrate. X-ray diffraction studies confirmed a good structural quality of our multilayers. The samples were characterised with vibrating sample magnetometer, longitudinal magnetooptical Kerr effect and giant magnetoresistance measurements. It was determined that our multilayers are magnetically very soft with Hc approx 1 Oe and show uniaxial anisotropy with HK approx 5 Oe. For gold sublayer thickness dAu close to 1.1 nm the antiferromagnetic coupling is present in very narrow Au thickness range (approx 0.2 nm). Despite a good structural quality of samples relatively small giant magnetoresistance value (1.2% at room temperature) was found. It is due to non-perfect aniferromagnetic coupling caused by pinholes.
 
PACS numbers: 75.70.-i, 75.70.Pa, 68.55.-a
 
INFLUENCE OF TEMPERATURE AND ANNEALING ON GMR IN SPUTTERED PERMALLOY/Cu MULTILAYERS

M. Urbaniaka, F. Stobieckia, T. Lucińskia, M. Kopcewiczb, A. Grabiasb and J. Aleksiejewa

a Institute of Molecular Physics, Polish Academy of Sciences Smoluchowskiego 17, 60-179 Poznań, Poland
b Institute of Electronic Materials Technology Wólczyńska 133, 01-919 Warszawa, Poland

The influence of temperature and annealing on giant magnetoresistance of Si(100)/Cu(20 nm)/Py(2 nm)/(Cu(2 nm)/Py(2 nm))100 multilayer (Py = Ni83Fe17) sputtered at room temperature in double face-to-face configuration is reported. It was found that giant magnetoresistance value, Delta RGMR/Rsat (where Rsat is the resistance in saturation), monotonically decreases with increasing temperature (4.5% at 173 K to about 1% at 373 K). This results from the decrease in magnetic change of resistance, Delta RGMR, and to the lesser extent from an increase in Rsat, though both of them are caused by the shortening of electrons mean free path. The observed almost linear decrease in giant magnetoresistance saturation field with increasing temperature is explained by temperature changes of magnetization profile. Vibrating sample magnetometer measurements revealed that the increase in temperature results in pronounced decrease in remnant to saturation magnetization ratio (Mr/Ms) suggesting that at low temperatures magnetic bridges between Py layers play an important role in magnetization process. It is shown that proper annealing, by an annihilation of bridges and/or lateral decoupling, leads to an increase in giant magnetoresistance ratio from 3.4% in as deposited state to 4.7%.
 
PACS numbers: 75.70.Ak, 75.70.Pa
 
MAGNETIC CHARACTERISTICS OF THE SYSTEM OF EXCHANGE COUPLED LAYERS

A. Urbaniak-Kucharczyk and S. Machowski

Department of Solid State Physics, University of Lódz Pomorska 149/153, 90-236 Lódz, Poland

Using the Green function method it is shown that the deviation of the Curie temperature from its value calculated for continuous layers is related to the absolute value of the interlayer coupling parameter. The dependence of spin wave stiffness parameter on the interlayer exchange coupling is also found.
 
PACS numbers: 75.70.Ak, 75.30.-m, 75.40.Cx
 
STM IMAGING OF MAGNETIC DOTS WITH FERROMAGNETIC TIP

A. Wawroa,b and A. Kasuyab

a Institute of Physics, Polish Academy of Sciences Al. Lotników 32/46, 02-668 Warsaw, Poland ^bInstitute for Materials Research, Tohoku University 2-1-1 Katahira, 980 Sendai, Japan

We report on imaging of isolated, few nanometers in size, magnetic dots (Co, Ni) by the use of a scanning tunneling microscope equipped with a ferromagnetic Co tip in the presence of external magnetic field. The dependence of apparent height of dots as a function of magnetic field takes a hysteresis-like shape. We discuss possible mechanisms of the scanning tunneling microscope tip interactions with dots.
 
PACS numbers: 34.80.Nz, 36.40.Cg, 61.16.Ch
 
STRUCTURAL STUDIES OF Co/Cu AND Co/Ru INTERFACES USING ^{59}Co NMR METHOD

M. Wójcik, E. Jedryka, S. Nadolski

Institute of Physics, Polish Academy of Sciences Al. Lotników 32/46, 02-668 Warszawa, Poland

D. Kubinski, M. Parsons and H. Holloway

Ford Research Laboratory, SRL/MD3028, Dearborn, MI 48121-2053, USA

The structural and magnetic properties of three magnetron sputtered multilayers at the 2nd maximum of antiferromagnetic coupling were studied using 59Co NMR spectroscopy: [Co(20 Ć)/Cu(20 Ć)]20, [Co(20 Ć )/ Ru(18 Ć)]20 and a heterostructure, in which non-magnetic spacers alternated between Cu and Ru. Co/Cu interfaces were found to be relatively sharp, extended over 3 monolayers, while the Co/Ru interfaces extend over 6 monolayers due to the good miscibility of Co and Ru. The NMR restoring field in the heterostructure is found to be the average of the restoring fields in both reference samples.
 
PACS numbers: 76.60.Lz, 75.70.Pa, 75.70.Cn, 75.20.En
 
PERPENDICULAR AND PARALLEL TRANSPORT, AND INTERLAYER EXCHANGE COUPLING IN MAGNETIC TRILAYERS WITH EXTRA CAP-LAYERS \aut {S. Krompiewski and M. Zwierzycki Institute of Molecular Physics, Polish Academy of Sciences Smoluchowskiego 17, 60-179 Poznań, Poland

Oscillations of magnetoresistance and interlayer exchange coupling vs. both non-magnetic spacer and cap-layer thicknesses are studied within the framework of the s-d model. The studies are carried out by means of the Kubo formula and a Green function recursion technique. Transport calculations concern multilayers (sandwiched between two semi-infinite ideal lead wires) oriented either parallel or perpendicular to the current direction. The considered structures for the above mentioned two basic geometries, are cubic grains identical in: (i) size, (ii) number of sublayers, and (iii) thicknesses of particular sublayers, which makes it possible to compare, in a direct and reliable way, the corresponding magnetoresistances. The current-in-plane magnetoresistance is found to be usually lower than the current-perpendicular-to-plane one, but both of them show oscillatory behaviours mutually correlated, and related to the Fermi surface callipers. Moreover, the current-perpendicular-to-plane giant magnetoresistance for structures in a form of infinite in layer-plane trilayers capped with an extra bilayer (ferromagnet/paramagnet) is also discussed.
 
PACS numbers: 75.70.-i, 75.70.Pa, 73.23.Ad
 
INELASTIC NEUTRON SCATTERING IN gamma-Mn(12%Ge) ALLOY ABOVE AND BELOW THE NÉEL TEMPERATURE

J. Jankowska-Kisielińskaa, K. Mikkea and B. Hennionb

a Institute of Atomic Energy, Swierk, 05-400 Otwock, Poland
bLaboratoire Lèon Brillouin, CEN Saclay, France

The magnetic excitations different from spin waves in the gamma-Mn(12%Ge) antiferromagnet are the subject of the present investigation. The inelastic neutron scattering was measured at 4 temperatures above TN. The Lorentzian-type formula for the inelastic neutron scattering cross-section with the spectral width for a hydrodynamic region was used for data analysis. The obtained values of the ``stiffness constants'' are of the order of 200 meV Ć\ and they depend weakly on temperature in the range of 1.04-1.25TN. The inelastic neutron scattering for energy transfers below and close to the value of the gap energy of the spin wave spectrum was measured at room temperature. The observed intensities can be treated as a sum of intensities of neutrons scattered on spin waves around the magnetic Brillouin zone centre and = those scattered on fluctuations at the zone boundary.
 
PACS numbers: 75.40.Gb, 75.30.Ds, 75.20.En
 
THE ENERGY SPECTRUM OF SINGLE-HOLE STATES IN TRANSITION METAL OXIDES

A. Lehmann-Szweykowskaa, R.J. Wojciechowskia and G.A. Gehringb

a Institute of Physics, A. Mickiewicz Univeresity, Umultowska 85, 61-614 Poznań, Poland
b Department of Physics and Astronomy, University of Sheffield, Sheffield S3 7RH, U.K.

The p-d hybridised single-hole states of the transition-metal-oxygen tetrahedron (TMO4) are collectivised due to the direct p-p hopping between oxygens of different clusters. The lowest-lying energy band is always narrow and fully occupied. The first excited band gets occupied as an effect of valence-uncompensated doping, so it can be almost localised. The possible hole excitations to the two higher energy bands, which are wider, may imply the Mott-like hopping form of charge transport in these systems.
 
PACS numbers: 71.10.Fd, 72.20.-i
 
EFFECTS OF CORE-HOLE SCREENING ON SPIN-POLARISED AUGER SPECTRA FROM FERROMAGNETIC Ni

T. Wegner, M. Potthoff and W. Nolting

Lehrstuhl ``Festkörpertheorie'', Institut für Physik, Humboldt-Universität zu Berlin Invalidenstraße 110, 10115 Berlin, Germany

We calculate the spin- and temperature-dependent local density of states for ferromagnetic Ni in the presence of a core hole at a distinguished site in the lattice. Correlations among the valence electrons and between valence and core electrons are described within a multi-band Hubbard model which is treated by means of second-order perturbation theory around the Hartree-Fock solution. The core-hole potential causes strong screening effects in the Ni valence band. The local magnetic moment is found to be decreased by a factor of 5-6. The consequences for the spin polarisation of CVV Auger electrons are discussed.
 
PACS numbers: 79.20.Fv, 71.20.Be, 75.60.Ej
 
MAGNETIC PROPERTIES OF SPIN-LADDERS (A2Cu2O3)m (CuO2)n

M. Barana, H. Szymczaka, R. Szymczaka, S. Dyeyeva, L. Leonyukb and G.-J. Babonasc

a Institute of Physics, Polish Academy of Sciences Al. Lotników 32/46, 02-668 Warsaw, Poland ^bMoscow State University, 119899 Moscow, Russian Federation
c Semiconductor Physics Institute, 2600 Vilnius, Lithuania

Magnetization M(T) and M(H) data of single crystals of the S=1/2 quasi-one-dimensional system (A2Cu2O3)m(CuO2)n with various A-site constituents are compared. The studied orthorhombic, incommensurate crystals are characterized by m/n=5/7,7/10, and 9/13. The role of rare-earth ions located in A-sites is discussed.
 
PACS numbers: 75.40.Cx, 75.30.Gw, 75.45.+j, 75.90.+w
 
THE MAGNETIC PROPERTIES AND THE BARKHAUSEN NOISE OF THE ANNEALED Fe-V-B AMORPHOUS ALLOY

L. Cenigaa, L. Novákb and A. Zentkoa

a Institute of Experimental Physics, Slovak Academy of Sciences Watsonova 47, 043 53 Ko\v sice, Slovak Republic ^bDepartment of Physics, Technical University Komenského park 2, 041 20 Kosice, Slovak Republic

As a consequence of the annealing process, the study of structural changes which can be followed by measuring structure sensitive magnetic properties as the stress induced anisotropy, the coercive force, the demagnetizing factor, and the Barkhausen noise parameters of the as-cast and annealed Fe80V5B15 amorphous alloys was performed. The structural changes were connected with the temperature range where the Fe80V5B15 amorphous alloy was characterized by the soft magnetic properties.
 
PACS numbers: 61.43.Dq, 75.50.Kj, 75.60.Ej
 
EXPERIMENTAL STUDIES OF S=1 HEISENBERG PLANAR ANTIFERROMAGNETIC CHAIN Ni(C11H10N2O)2Ni(CN)4

E. Cizmára, J. Cernáka, M. Orendáca, T. Herrmannsdörferb and A. Fehera

a Faculty of Science, P.J. Safárik University, Park Angelinum 9, 04154 Ko\v sice, Slovakia
b Physikalisches Institut, Universität Bayreuth, 95440 Bayreuth, Germany

In this paper we discuss the results of experimental studies of specific heat and magnetic susceptibility of chain compound Ni(C11H10N2O)2Ni(CN)4. We have observed a Schottky type anomaly at T=2.2 K in a temperature dependence of specific heat and the compound was identified as a S=1 Heisenberg antiferromagnetic chain with the subcritical exchange coupling D/kB=5 K, D/|J|=5.2 and the strong in-plane anisotropy E/kB=2.8 K. It has been found that the in-plane anisotropy affects the region of validity of a diluted exciton model [1] and a strong coupling model [2] for S=1 Heisenberg chains with the strong planar anisotropy. The analysis suggests that the in-plane anisotropy should be considered in any attempt to find a compound potentially located in the boundary of Haldane and ``large-D'' phases.
 
PACS numbers: 75.40.Cx, 71.20.Be, 75.50.Ee
 
INFLUENCE OF THE LOCAL ENVIRONMENT ON THE MAGNETIC PROPERTIES OF THE ORDERED Fe1-xAlx ALLOY

J. Deniszczyk

Institute of Physics and Chemistry of Metals, Silesian University Bankowa 12, 40-007 Katowice, Poland

The electronic and magnetic properties of the ordered binary Fe1-xAlx alloy with the B2 crystal structure were calculated for Al concentrations x=0.1875-0.5 using the supercell structure. The calculations showed that for increasing Al contents the average magnetization of Fe1-xAlx falls down rapidly. Upon lowering the unit cell volume, almost all configurations of compositions with x >= 0.25 show the abrupt change of magnetic state from the high moment magnetic state to the low moment magnetic state with the moment reduction 0.6-0.8 ”B per atom. The configurations were found for which the low moment magnetic state solutions with the antiferromagnetic alignment of magnetic moments of Fe atoms at antisite positions are stable.
 
PACS numbers: 71.15.La, 71.15.Fv, 71.20.Lp, 75.50.Bb, 75.30.-m
 
MAGNETIC PROPERTIES OF FERROFLUID WITH COBALT FERRITE PARTICLES

P. Didukha, A. Slawska-Waniewskaa, J.M. Grenecheb and P.C. Fanninc

a Institute of Physics, Polish Academy of Sciences Al. Lotników 32/46, 02-668 Warsaw, Poland
b Laboratoire de Physique, UPRESA CNRS 6087, Université du Maine 72085 Le Mans, France
c Department of Electronic & Electrical Engineering, Trinity College Dublin 2, Ireland

Low temperature Mössbauer investigations of a diluted magnetic fluid containing ultrafine CoFe2O4 particles are presented. The thermal evolution of cobalt ferrite particles from the magnetically ordered state to the superparamagnetic state with the blocking temperature at about 80 K, is shown.
 
PACS numbers: 75.50.Mm, 76.80.+y, 61.18.Fs
 
AC SUSCEPTIBILITY MEASUREMENTS IN THE INVESTIGATION OF AGGREGATION IN MAGNETIC FLUIDS

P.C. Fannina and S.W. Charlesb

a Dept. of Electronic & Electrical Engineering, Trinity College Dublin 2, Ireland
b Dept. of Chemistry, University College of North Wales, Bangor, LL57 2UW, UK

Measurements of the complex, frequency dependent susceptibility, chi(omega)=chi '(omega)-ichi''(omega) of two water based magnetic fluids, over the frequency range 10 Hz to 1 MHz are reported. Plots of the susceptibility components against log[f(Hz)] are found to have approximate Debye-type profiles with the presence of Brownian relaxation being indicated by the frequency, fmax, of the maximum of the loss-peaks in the chi''(omega) profiles. Corresponding calculations of particle hydrodynamic radius indicate the presence of aggregation. Frohlich, normal and lognormal distribution functions are used to obtain an estimate of the aggregate size distribution in the samples.
 
PACS numbers: 75.50.Tt, 76.20.+q
 
JOULE HEATING PREANNEALING EFFECT IN THE COERCIVITY FIELD AND MAGNETOSTRICTION CONSTANT OF Co66Fe4Mo2Si16B12 ALLOY

P. Garcia Telloa, J. Gonzálezb, J.M. Blancoa and R. Zuberekc

a Dpto. Fisica Aplicada I, EUITI, San Sebastián, Spain
b Dpto. Fisica de Materiales, Facultad de CC Quimicas UPV, San Sebastián, Spain
c Institute of Physics, Polish Academy of Sciences Al. Lotników 32/46, 02-668 Warszawa, Poland

The effect of thermal treatments (by the Joule heating and conventional annealing) on the coercivity and saturation magnetostriction constant in the amorphous and nanocrystalline Co66Fe4Mo2Si16B12 alloy is reported. It is noticeable the near insensibility to the external stress of coercive field and anisotropy field (leading to extremely low value of magnetostriction 1.5Ś10^-8) achieved after the Joule heating by two steps (first one to relax the internal stresses and the second one to develop a fine nanocrystalline structure).
 
PACS numbers: 75.50.Kj, 75.30.Gw, 75.80.+q
 
MAGNETOELASTIC ANOMALIES AND SUPPRESSION OF JAHN-TELLER DISTORTIONS IN La1-xSrxMnO3 BY PULSED MAGNETIC FIELDS

A.M. Kadomtsevaa, Yu.F. Popova, G.P. Vorob'eva, K.I. Kamilova, V.Yu. Ivanovb, A.A. Mukhinb and A.M. Balbashovc

a Moscow State University, Leninskie Gori, 119899 Moscow, Russia
b General Physics Institute of the RAS, 38 Vavilov St., 117942 Moscow, Russia
c Moscow Power Engineering Inst., 14 Krasnokazarmen St., 105835 Moscow, Russia

Thermal expansion Delta l/l(T) and magnetostriction lambdaparallel,perp(H,T) in the pulsed magnetic fields H up to 250 kOe were studied in the single La1-xSrxMnO3 crystals (x=0.1, 0 .125, and 0.15) at temperatures T=10-320 K. Anomalies in the Delta l/l (T) curves were observed near a charge (polaron) ordering (Tp) and structural transitions between orthorhombic Jahn-Teller distorted O' phase and high temperature orthorhombic (pseudocubic) O* one (T's). A noticeable increase in the field-induced magnetostriction lambdaparallel,perp(H) was revealed in the O' phase at Tp<T<T's. Jumps in the lambdaparallel,perp(H) curves were observed at temperatures near Tp. The observed features may be related to a suppression of the Jahn-Teller O' phase by the magnetic field and field induced transition to a new orbital-ordered ferromagnetic state.
 
PACS numbers: 75.30.Kz, 75.50.Pp
 
XPS STUDY OF ``INFINITE CHAIN''
Ca2CuO3 AND Ca0.5Sr0.5CuO2 COMPOUNDS

I. Jacyna-Onyszkiewicza and Yu.B. Poltorackyb

a Institute of Physics, Adam Mickiewicz University Umultowska 85, 61-614 Poznań, Poland
b NMO ``Monocrystalreactiv'', Lenin 60, 310077 Kharkov, Ukraine

Al Kalpha excited photoelectron spectra (X-ray photoelectron spectroscopy) of the O 1s, Cu 2p, Ca 2p, Sr 3d core levels were measured for ``infinite chain'' Ca2CuO3 and Ca0.5Sr0.5CuO2 compounds. The analysis indicates that for Ca2CuO3 the surface electronic structure is strongly influenced by a humid atmosphere. The surface layer is formed predominantly by copper hydroxide. The minor features of Cu 2p and O 1s are characteristic of the bulk bonding states. The valences of the Cu, Ca, and Sr atoms are close to 2+. The core electron binding energies (\approx 934 eV peak) are due to the 2p3/23d10L1 configuration of Cu(II) ions in the square planar coordination for both samples.
 
PACS numbers: 79.60.-i, 74.72.-h, 74.72.Jt
 
INFLUENCE OF LOCAL ENVIRONMENT ON THE ELECTRONIC STRUCTURE AND MAGNETIC PROPERTIES OF Ni1-xCuxMnSb ALLOYS

A. Jezierskia and A. Szytulab

a Institute of Molecular Physics, Polish Academy of Sciences Smoluchowskiego 17, 60-179 Poznań, Poland
b Institute of Physics, Jagiellonian University, Reymonta 4, 30-059 Kraków, Poland

The magnetic ordering in Ni1-xCuxMnSb alloys changes from ferromagnetic (x=0) to antiferromagnetic (x=1). The X-ray and neutron diffraction showed that the systems crystallise in C1b type structure. We present an influence of the local chemical ordering on the electronic and magnetic properties of Ni1-xCuxMnSb alloys. The band structure and the magnetic moments were calculated by the spin-polarised linear muffin-tin orbital in the atomic sphere approximation method for the experimental values of the lattice parameters. The magnetic moment of Mn increases from 3.8 ”B for x=0 to 4.18 ”B for x=1.
 
PACS numbers: 31.15.Ar, 31.15.Ew, 71.15.Mb, 71.15.-m, 71.15.La, 71.20.-b, 71.20.Be
 
THE MAGNETIC PROPERTIES AND THE BARKHAUSEN NOISE OF THE HYDROGENATED Fe-V-B AMORPHOUS ALLOY

L. Cenigaa and L. Novákb

a Institute of Experimental Physics, Slovak Academy of Sciences Watsonova 47, 043 53 Kosice, Slovak Republic
b Department of Physics, Technical University Komenského park 2, 041 20 Ko\v sice, Slovak Republic

As a consequence of the hydrogenation-dehydrogenation process, in the present paper the study of structural changes which could be followed by measuring structure sensitive magnetic properties as the stress induced anisotropy, the coercive force, the demagnetizing factor, and the Barkhausen noise parameters of the as-cast and hydrogenated Fe80V5B15 amorphous alloys is performed.
 
PACS numbers: 61.43.Dq, 75.50.Kj, 75.60.Ej
 
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