PIPT from the Beginning to Future

H. Cailleaua,b, T. Lutyc, S. Koshiharab, M. Servola, M. Lorenca, M. Buron-Le Cointea and E. Colleta aInstitut de Physique de Rennes, Université de Rennes 1-CNRS, UMR 6251, Rennes, France, bJST, CREST and Department of Material Science, Tokyo Institute of Technology, Tokyo, Japan, cInstitute of Physical and Theoretical Chemistry, Wrocław University of Technology, Wrocław, Poland

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The birth of the field of photoinduced phase transitions was strongly influenced by the conceptual viewpoint expressed by Professor Y. Toyozawa on the condensation of relaxed excitons. Since this first period, twenty years ago, this young field has been expanding rapidly along a diversity of directions. Nowadays, it goes hand in hand with the challenges of today's science: emergence, nonlinearity, coherence, far away from equilibrium, for example. The control of the functionality of a material via photoexcited states poses many new fundamental questions. Some of them will be overviewed: (i) the nature of the control parameters and the nature of the relevant collective variables, especially the order parameters, which characterize the evolution of the system, (ii) the difference between photoinduced transformations under continuous light irradiation and those resulting from an ultrashort laser pulse, (iii) the physical mechanisms of ultrafast photoinduced phase transitions from the formation and proliferation of phototransformed entities to the softening of a collective mode.

DOI: 10.12693/APhysPolA.121.297 PACS numbers: 64.60.-i, 64.70.K-, 78.47.D-